http://www.pnas.org/content/110/40/15908.abstract

Wright, J. D. & Schaller, M. F., 2013: Evidence for a rapid release of carbon at the Paleocene-Eocene thermal maximum.

–Proceedings of the National Academy of Sciences: Vol. 110, #40, pp. 15908- 15913 [doi: 10.1073/pnas.1309188110]

Abstract

The Paleocene/Eocene thermal maximum (PETM) and associated carbon isotope excursion (CIE) are often touted as the best geologic analog for the current anthropogenic rise in pCO_2. However, a causal mechanism for the PETM CIE remains unidentified because of large uncertainties in the duration of the CIE’s onset. Here, we report on a sequence of rhythmic sedimentary couplets comprising the Paleocene/Eocene Marlboro Clay (Salisbury Embayment). These couplets have corresponding δ¹⁸O cycles that imply a climatic origin. Seasonal insolation is the only regular climate cycle that can plausibly account for δ¹⁸O amplitudes and layer counts. High-resolution stable isotope records show 3.5‰ δ¹³C decrease over 13 couplets defining the CIE onset, which requires a large, instantaneous release of ¹³C-depleted carbon. During the CIE, a clear δ¹³C gradient developed on the shelf with the largest excursions in shallowest waters, indicating atmospheric δ¹³C decreased by ∼20‰. Our observations and revised release rate are consistent with an atmospheric perturbation of 3,000-gigatons of carbon (GtC).